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Moussa Abu Marzouk told The Associated Press in an interview that Hamas "did not close and will not close the door until we release our prisoners from Israeli jails."
Egyptian-brokered talks over a deal that would see Israel release hundreds of Palestinian prisoners in exchange for Schalit broke down last week.
Prime Minister Ehud Olmert said early this week that Hamas' excessive demands prevented the deal and indicated he would turn the matter over to his successor, Binyamin Netanyahu.